Unleashing the Full Sustainable Potential of Thick Films of Lead-Free Potassium Sodium Niobate (K0.5Na0.5NbO3) by Aqueous Electrophoretic Deposition

A current challenge for the fabrication of functional oxide-based devices is related with the need of environmental and sustainable materials and processes. By considering both lead-free ferroelectrics of potassium sodium niobate (K0.5Na0.5NbO3, KNN) and aqueous-based electrophoretic deposition here...

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Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1992. - 32(2016), 21 vom: 31. Mai, Seite 5241-9
1. Verfasser: Mahajan, Amit (VerfasserIn)
Weitere Verfasser: Pinho, Rui, Dolhen, Morgane, Costa, M Elisabete, Vilarinho, Paula M
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2016
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article Research Support, Non-U.S. Gov't
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520 |a A current challenge for the fabrication of functional oxide-based devices is related with the need of environmental and sustainable materials and processes. By considering both lead-free ferroelectrics of potassium sodium niobate (K0.5Na0.5NbO3, KNN) and aqueous-based electrophoretic deposition here we demonstrate that an eco-friendly aqueous solution-based process can be used to produce KNN thick coatings with improved electromechanical performance. KNN thick films on platinum substrates with thickness varying between 10 and 15 μm have a dielectric permittivity of 495, dielectric losses of 0.08 at 1 MHz, and a piezoelectric coefficient d33 of ∼70 pC/N. At TC these films display a relative permittivity of 2166 and loss tangent of 0.11 at 1 MHz. A comparison of the physical properties between these films and their bulk ceramics counterparts demonstrates the impact of the aqueous-based electrophoretic deposition (EPD) technique for the preparation of lead-free ferroelectric thick films. This opens the door to the possible development of high-performance, lead-free piezoelectric thick films by a sustainable low-cost process, expanding the applicability of lead-free piezoelectrics 
650 4 |a Journal Article 
650 4 |a Research Support, Non-U.S. Gov't 
700 1 |a Pinho, Rui  |e verfasserin  |4 aut 
700 1 |a Dolhen, Morgane  |e verfasserin  |4 aut 
700 1 |a Costa, M Elisabete  |e verfasserin  |4 aut 
700 1 |a Vilarinho, Paula M  |e verfasserin  |4 aut 
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