Construction of a Semiconductor-Biological Interface for Solar Energy Conversion : p-Doped Silicon/Photosystem I/Zinc Oxide

The interface between photoactive biological materials with two distinct semiconducting electrodes is challenging both to develop and analyze. Building off of our previous work using films of photosystem I (PSI) on p-doped silicon, we have deposited a crystalline zinc oxide (ZnO) anode using confine...

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Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1992. - 31(2015), 36 vom: 15. Sept., Seite 10002-7
1. Verfasser: Beam, Jeremiah C (VerfasserIn)
Weitere Verfasser: LeBlanc, Gabriel, Gizzie, Evan A, Ivanov, Borislav L, Needell, David R, Shearer, Melinda J, Jennings, G Kane, Lukehart, Charles M, Cliffel, David E
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2015
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article Research Support, Non-U.S. Gov't Research Support, U.S. Gov't, Non-P.H.S. Photosystem I Protein Complex Zinc Oxide SOI2LOH54Z Silicon Z4152N8IUI
Beschreibung
Zusammenfassung:The interface between photoactive biological materials with two distinct semiconducting electrodes is challenging both to develop and analyze. Building off of our previous work using films of photosystem I (PSI) on p-doped silicon, we have deposited a crystalline zinc oxide (ZnO) anode using confined-plume chemical deposition (CPCD). We demonstrate the ability of CPCD to deposit crystalline ZnO without damage to the PSI biomaterial. Using electrochemical techniques, we were able to probe this complex semiconductor-biological interface. Finally, as a proof of concept, a solid-state photovoltaic device consisting of p-doped silicon, PSI, ZnO, and ITO was constructed and evaluated
Beschreibung:Date Completed 08.07.2016
Date Revised 15.09.2015
published: Print-Electronic
Citation Status MEDLINE
ISSN:1520-5827
DOI:10.1021/acs.langmuir.5b02334