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231224s2015 xx |||||o 00| ||eng c |
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|a 10.1021/la503776b
|2 doi
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|a pubmed24n0816.xml
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|c DE-627
|e rakwb
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|a eng
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| 100 |
1 |
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|a Shah, Vivek B
|e verfasserin
|4 aut
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| 245 |
1 |
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|a Linker-free deposition and adhesion of Photosystem I onto nanostructured TiO2 for biohybrid photoelectrochemical cells
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|c 2015
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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| 500 |
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|a Date Completed 29.02.2016
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|a Date Revised 10.02.2015
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|a published: Print-Electronic
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|a Citation Status MEDLINE
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|a Photosystem I (PSI) from oxygenic photosynthetic organisms is an attractive sensitizer for nano-biohybrid solar cells as it has a combined light-harvesting and reaction center in one protein complex and operates at a quantum yield close to one in biological systems. Using a linker-free deposition technique enabled by an electrospray system, PSI was coupled to 1-D nanostructured titanium dioxide thin films to fabricate an electrode for a photoelectrochemical cell. After deposition, the surfactant in the PSI aggregate was dissolved in the surfactant-free electrolyte, ensuring that partly hydrophobic PSI was not resuspended and stayed in contact with titanium dioxide. A maximum current density of 4.15 mA cm(-2) was measured after 10 min of electrospray deposition, and this is the highest current density reported so far for PSI-based photoelectrochemical cells. The high current is attributed to 1D nanostructure of titanium dioxide and orientation of the PSI onto the surface, which allows easy transfer of electrons
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|a Journal Article
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|a Research Support, Non-U.S. Gov't
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|a Research Support, U.S. Gov't, Non-P.H.S.
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|a Photosystem I Protein Complex
|2 NLM
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|a titanium dioxide
|2 NLM
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|a 15FIX9V2JP
|2 NLM
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|a Titanium
|2 NLM
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|a D1JT611TNE
|2 NLM
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| 700 |
1 |
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|a Henson, William R
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Chadha, Tandeep S
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Lakin, Gerard
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Liu, Haijun
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Blankenship, Robert E
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Biswas, Pratim
|e verfasserin
|4 aut
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| 773 |
0 |
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1992
|g 31(2015), 5 vom: 10. Feb., Seite 1675-82
|w (DE-627)NLM098181009
|x 1520-5827
|7 nnns
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| 773 |
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|g volume:31
|g year:2015
|g number:5
|g day:10
|g month:02
|g pages:1675-82
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|u http://dx.doi.org/10.1021/la503776b
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