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231224s2013 xx |||||o 00| ||eng c |
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|a 10.1021/la400177u
|2 doi
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|a pubmed24n0756.xml
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|a (NLM)23594344
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|a DE-627
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|e rakwb
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|a eng
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|a Makarova, Marina
|e verfasserin
|4 aut
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|a Ordered monomolecular layers as a template for the regular arrangement of gold nanoparticles
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|c 2013
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 06.01.2014
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|a Date Revised 18.06.2013
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|a published: Print-Electronic
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|a Citation Status MEDLINE
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|a Ordered arrays of metal nanoparticles are important for nanoelectronic and nanophotonic applications. Here, we report the formation of self-assembled arrays of gold nanoparticles on molecular layers of diacetylene compounds on a MoS2(0001) substrate. The arrangement of gold nanoparticles is observed using scanning tunneling microscopy. When gold is deposited on a self-assembled monolayer of 10,12-nonacosadiynoic acid or 10,12-octadecadiynoic acid on a MoS2(0001) substrate, the ordered array of diacetylene moieties in the molecular layer serves as a template for the formation of ordered arrays of gold nanoparticles. In contrast, when gold is deposited on a pristine MoS2(0001) surface or on a molecular layer of stearic acid, the gold nanoparticles are randomly distributed on the surface. It is found that the arrangement of gold nanoparticles is largely determined by the deposition rate; faster deposition results in more ordered arrays of gold nanoparticles. Our observations confirm the role of unsaturated π systems in molecules acting as a template for the regular arrangement of gold nanoparticles; this work will open up new possibilities for interfacial nanoarchitectonics
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|a Journal Article
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|a Research Support, Non-U.S. Gov't
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|a Gold
|2 NLM
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|a 7440-57-5
|2 NLM
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|a Mandal, Swapan K
|e verfasserin
|4 aut
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|a Okawa, Yuji
|e verfasserin
|4 aut
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|a Aono, Masakazu
|e verfasserin
|4 aut
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1992
|g 29(2013), 24 vom: 18. Juni, Seite 7334-43
|w (DE-627)NLM098181009
|x 1520-5827
|7 nnns
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|g volume:29
|g year:2013
|g number:24
|g day:18
|g month:06
|g pages:7334-43
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|u http://dx.doi.org/10.1021/la400177u
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