Structure determination of Pt-coated Au dumbbells via fluctuation X-ray scattering

A fluctuation X-ray scattering experiment has been carried out on platinum-coated gold nanoparticles randomly oriented on a substrate. A complete algorithm for determining the electron density of an individual particle from diffraction patterns of many particles randomly oriented about a single axis...

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Détails bibliographiques
Publié dans:Journal of synchrotron radiation. - 1994. - 19(2012), Pt 5 vom: 05. Sept., Seite 695-700
Auteur principal: Chen, Gang (Auteur)
Autres auteurs: Modestino, Miguel A, Poon, Billy K, Schirotzek, André, Marchesini, Stefano, Segalman, Rachel A, Hexemer, Alexander, Zwart, Peter H
Format: Article en ligne
Langue:English
Publié: 2012
Accès à la collection:Journal of synchrotron radiation
Sujets:Journal Article Research Support, U.S. Gov't, Non-P.H.S.
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520 |a A fluctuation X-ray scattering experiment has been carried out on platinum-coated gold nanoparticles randomly oriented on a substrate. A complete algorithm for determining the electron density of an individual particle from diffraction patterns of many particles randomly oriented about a single axis is demonstrated. This algorithm operates on angular correlations among the measured intensity distributions and recovers the angular correlation functions of a single particle from measured diffraction patterns. Taking advantage of the cylindrical symmetry of the nanoparticles, a cylindrical slice model is proposed to reconstruct the structure of the nanoparticles by fitting the experimental ring angular auto-correlation and small-angle scattering data obtained from many scattering patterns. The physical meaning of the refined structure is discussed in terms of their statistical distributions of the shape and electron density profile 
650 4 |a Journal Article 
650 4 |a Research Support, U.S. Gov't, Non-P.H.S. 
700 1 |a Modestino, Miguel A  |e verfasserin  |4 aut 
700 1 |a Poon, Billy K  |e verfasserin  |4 aut 
700 1 |a Schirotzek, André  |e verfasserin  |4 aut 
700 1 |a Marchesini, Stefano  |e verfasserin  |4 aut 
700 1 |a Segalman, Rachel A  |e verfasserin  |4 aut 
700 1 |a Hexemer, Alexander  |e verfasserin  |4 aut 
700 1 |a Zwart, Peter H  |e verfasserin  |4 aut 
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