Fast, high-throughput creation of size-tunable micro/nanoparticle clusters via evaporative self-assembly in picoliter-scale droplets of particle suspension

We report a fast, high-throughput method to create size-tunable micro/nanoparticle clusters via evaporative assembly in picoliter-scale droplets of particle suspension. Mediated by gravity force and surface tension force of a contacting surface, picoliter-scale droplets of the suspension are generat...

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Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1992. - 28(2012), 6 vom: 14. Feb., Seite 3102-11
1. Verfasser: Choi, Sun (VerfasserIn)
Weitere Verfasser: Jamshidi, Arash, Seok, Tae Joon, Wu, Ming C, Zohdi, Tarek I, Pisano, Albert P
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2012
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article
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520 |a We report a fast, high-throughput method to create size-tunable micro/nanoparticle clusters via evaporative assembly in picoliter-scale droplets of particle suspension. Mediated by gravity force and surface tension force of a contacting surface, picoliter-scale droplets of the suspension are generated from a nanofabricated printing head. Rapid evaporative self-assembly of the particles on a hydrophobic surface leads to fast clustering of micro/nanoparticles and forms particle clusters of tunable sizes and controlled spacing. The evaporating behavior of the droplet is observed in real-time, and the clustering characteristics of the particles are understood based on the physics of evaporative-assembly. With this method, multiplex printing of various particle clusters with accurate positioning and alignment are demonstrated. Also, size-unifomity of the cluster arrays is thoroughly analyzed by examining the metallic nanoparticle cluster-arrays based on surface-enhanced Raman spectroscopy (SERS) 
650 4 |a Journal Article 
700 1 |a Jamshidi, Arash  |e verfasserin  |4 aut 
700 1 |a Seok, Tae Joon  |e verfasserin  |4 aut 
700 1 |a Wu, Ming C  |e verfasserin  |4 aut 
700 1 |a Zohdi, Tarek I  |e verfasserin  |4 aut 
700 1 |a Pisano, Albert P  |e verfasserin  |4 aut 
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