Preparation of raspberry-like nanocapsules by the combination of Pickering emulsification and solvent displacement technique

Well-defined raspberry-like nanocapsules were prepared by the combination of Pickering emulsification and solvent displacement technique by using silica particles as stabilizer and hexadecane (HD) as soft template. The formation of the capsule morphology is caused by the phase separation of poly(sty...

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Détails bibliographiques
Publié dans:Langmuir : the ACS journal of surfaces and colloids. - 1985. - 27(2011), 11 vom: 07. Juni, Seite 6689-700
Auteur principal: Schrade, Anika (Auteur)
Autres auteurs: Cao, Zhihai, Landfester, Katharina, Ziener, Ulrich
Format: Article en ligne
Langue:English
Publié: 2011
Accès à la collection:Langmuir : the ACS journal of surfaces and colloids
Sujets:Journal Article
Description
Résumé:Well-defined raspberry-like nanocapsules were prepared by the combination of Pickering emulsification and solvent displacement technique by using silica particles as stabilizer and hexadecane (HD) as soft template. The formation of the capsule morphology is caused by the phase separation of poly(styrene-co-4-vinyl pyridine) (poly(St-co-4-VP)) in the droplets due to the diffusion of good solvent for the (co)polymer to the aqueous continuous phase. The size of capsules was successfully reduced from tens of micrometers in the dispersion by simply stirring to the nanorange by the employment of sonication and Ostwald ripening. The formation of silica-particles-armored nanocapsules was confirmed by transmission electron microscopy (TEM), high-resolution scanning electron microscopy (HRSEM), dynamic light scattering (DLS), and zeta potential measurement. The colloidal stability and particle properties, including size and morphology, depend on the amount of HD, and copolymers, the sonication time, the dispersion pH value, the type of solvent, and the copolymer composition
Description:Date Completed 23.09.2011
Date Revised 31.05.2011
published: Print-Electronic
Citation Status PubMed-not-MEDLINE
ISSN:1520-5827
DOI:10.1021/la201170w