Facile subsequently light-induced route to highly efficient and stable sunlight-driven Ag-AgBr plasmonic photocatalyst

In this paper, we successfully fabricate a stable and highly efficient direct sunlight plasmonic photocatalyst Ag-AgBr through a facile hydrothermal and subsequently sunlight-induced route. The diffuse reflectance spectra of Ag-AgBr indicate strong absorption in both UV and visible light region. The...

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Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1992. - 26(2010), 24 vom: 21. Dez., Seite 18723-7
1. Verfasser: Kuai, Long (VerfasserIn)
Weitere Verfasser: Geng, Baoyou, Chen, Xiaoting, Zhao, Yanyan, Luo, Yinchan
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2010
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article Research Support, Non-U.S. Gov't Bromides Silver Compounds Silver 3M4G523W1G silver bromide NHQ37BJZ2Z
Beschreibung
Zusammenfassung:In this paper, we successfully fabricate a stable and highly efficient direct sunlight plasmonic photocatalyst Ag-AgBr through a facile hydrothermal and subsequently sunlight-induced route. The diffuse reflectance spectra of Ag-AgBr indicate strong absorption in both UV and visible light region. The obtained photocatalyst shows excellent sunlight-driven photocatalytic performance. It can decompose organic dye within several minutes under direct sunlight irradiation and maintain a high level even though used five times. In addition, both the scanning electron microscopy images and X-ray photoelectron spectroscopy dates reveal the as-prepared photocatalyst to be very stable. Moreover, the mechanism suggests that the high photocatalytic activity and excellent stability result from the super sensitivity of AgBr to light, the surface plasmon resonance of Ag nanoparticles in the region of visible light, and the complexation between Ag(+) and nitrogen atom. Thus, the facile preparation and super performance of Ag-AgBr will make it available to utilize sunlight efficiently to remove organic pollutants, destroy bacteria, and so forth
Beschreibung:Date Completed 17.03.2011
Date Revised 21.11.2013
published: Print-Electronic
Citation Status MEDLINE
ISSN:1520-5827
DOI:10.1021/la104022g