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231223s2010 xx |||||o 00| ||eng c |
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|a 10.1021/la1034036
|2 doi
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|a eng
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|a Li, Le-Le
|e verfasserin
|4 aut
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|a Hierarchical self-assembly of superlattice hybrids consisting of periodic and alternating cores of porphyrin molecules separated by nanoscale silica walls
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|c 2010
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 21.01.2011
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|a Date Revised 12.10.2010
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|a published: Print
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|a Citation Status PubMed-not-MEDLINE
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|a Molecularly engineered superlattice hybrids consisting of periodic and alternating cores of porphyrin molecules separated by nanoscale silica walls were synthesized through a one-step organic-inorganic hierarchical self-assembly approach. The self-assembly process not only could lock both porphyrin and inorganic building blocks into ordered 3D nanostructure but also could allow for the molecular-level controllable organization of porphyrin molecules in the central regions of the silica pore channels, which leads to the formation of porphyrin core-silica wall superlattice hybrids with molecular-scale and mesoscale ordering. It was demonstrated that both the mesostructure and morphology of the hybrids can be finely tailored by turning the cooperative self-assembly process. It is significant that the hybrids show self-assembled optical properties consistent with the orientational arrangement of the porphyrins within periodic nanoscale silica channels. The methodology introduced herein demonstrates high versatility with respect to the self-assembly of optical active macrocycles into highly ordered superlattice hybrid architectures
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|a Journal Article
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|a Fu, Xue-Feng
|e verfasserin
|4 aut
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1 |
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|a Ren, Zhen
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhao, Ya-Guang
|e verfasserin
|4 aut
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| 700 |
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|a Feng, Wei
|e verfasserin
|4 aut
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| 700 |
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|a Yan, Chun-Hua
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1985
|g 26(2010), 20 vom: 19. Okt., Seite 15730-3
|w (DE-627)NLM098181009
|x 1520-5827
|7 nnns
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| 773 |
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|g volume:26
|g year:2010
|g number:20
|g day:19
|g month:10
|g pages:15730-3
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|u http://dx.doi.org/10.1021/la1034036
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