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231223s2010 xx |||||o 00| ||eng c |
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|a 10.1021/la102963w
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|a eng
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| 100 |
1 |
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|a Jin, Haibao
|e verfasserin
|4 aut
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| 245 |
1 |
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|a Polymerization-like multilevel hierarchical self-assembly of polymer vesicles into macroscopic superstructures with controlled complexity
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| 264 |
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|c 2010
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| 336 |
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|a Text
|b txt
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|a ƒaComputermedien
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|a Date Completed 04.01.2011
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|a Date Revised 14.09.2010
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|a published: Print
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|a Citation Status PubMed-not-MEDLINE
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|a We demonstrate a high-leveled hierarchical self-assembly process into fractal structures. Two hyperbranched multiarm copolymers are first coassembled into binary isotropic vesicles in the primary self-assembly. Then, these primary vesicles are in situ endowed with anisotropic hydrophobic "binding sites" through a pH-induced lateral microphase separation, undergoing an isotropic-anisotropic transition. Subsequently, the anisotropic vesicles further assemble together through the specific self-recognition between the binding sites into linear, branched, cyclization, and network-like vesicle chains. Furthermore, the obtained vesicle chains can transform into linear, branched, ring-like, and network tubes through successive vesicle fusion. Such a hierarchical process is pH-triggered and well-controlled by adjusting the vesicle compositions and is coined as "polymerization-like" self-assembly due to the striking analogy between the vesicle association model and polymerization process
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|a Journal Article
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|a Zhou, Yongfeng
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Huang, Wei
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Yan, Deyue
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1991
|g 26(2010), 18 vom: 21. Sept., Seite 14512-9
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