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231223s2008 xx |||||o 00| ||eng c |
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|a 10.1021/la800670b
|2 doi
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|a eng
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| 100 |
1 |
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|a Faulkner, Christopher J
|e verfasserin
|4 aut
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| 245 |
1 |
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|a Rapid assembly of photosystem I monolayers on gold electrodes
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|c 2008
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Completed 17.09.2008
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|a Date Revised 13.08.2008
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a Photosystem I (PSI) has drawn widespread interest for use in biomimetically inspired energy conversion devices upon extracting it from plants or cyanobacteria and assembling it at surfaces. Here, we demonstrate that a critically dense monolayer of spinach-derived PSI must be formed on an electrode surface to achieve optimal photocurrents, and we introduce a new method for preparing these dense PSI monolayers that reduces the time required for assembly by approximately 80-fold in comparison to that for adsorption from solution. This method consists of applying a vacuum above the aqueous PSI solution during assembly to concentrate PSI and precipitate it into a thick layer onto the surface of various self-assembled monolayers or directly onto the electrode surface. Rinsing with water yields a dense monolayer of PSI that draws approximately 100 nA/cm2 of light-induced current from the gold electrode in the presence of appropriate mediators
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|a Journal Article
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1 |
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|a Lees, Susan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Ciesielski, Peter N
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Cliffel, David E
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Jennings, G Kane
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1992
|g 24(2008), 16 vom: 19. Aug., Seite 8409-12
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