Influence of amphiphilic block copolymers on lyotropic liquid crystals in water-oil-surfactant systems

In ternary water-oil-nonionic alkyl polyglycol ether (C(i)E(j)) microemulsions, an increase in efficiency is always accompanied by the formation of a lamellar (L(alpha)) phase. The addition of an amphiphilic block copolymer to the ternary base system increases the efficiency of the microemulsion dra...

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Publié dans:Langmuir : the ACS journal of surfaces and colloids. - 1985. - 21(2005), 20 vom: 27. Sept., Seite 9058-67
Auteur principal: Frank, Christian (Auteur)
Autres auteurs: Sottmann, Thomas, Stubenrauch, Cosima, Allgaier, Jürgen, Strey, Reinhard
Format: Article
Langue:English
Publié: 2005
Accès à la collection:Langmuir : the ACS journal of surfaces and colloids
Sujets:Journal Article
Description
Résumé:In ternary water-oil-nonionic alkyl polyglycol ether (C(i)E(j)) microemulsions, an increase in efficiency is always accompanied by the formation of a lamellar (L(alpha)) phase. The addition of an amphiphilic block copolymer to the ternary base system increases the efficiency of the microemulsion drastically while suppressing--at least partly--the formation of the L(alpha) phase. However, amphiphilic block copolymers can be used not only to suppress the formation of lyotropic liquid crystals but also for the opposite effect, namely, to induce their formation. To understand to what extent the increase in efficiency is accompanied by the formation of lyotropic liquid crystals, we studied phase diagrams of water-n-alkane-n-alkyl polyglycol ethers (C(i)E(j))-PEPX-PEOY at a constant volume fraction of oil in the water/oil mixture. Using polymers of the poly(ethylene propylene)-copoly(ethylene oxide) type, with M(PEP) = X kg mol(-1) and M(PEO) = Y kg mol(-1), we determined phase diagrams as a function of the polymer concentration, size, and symmetry. Moreover, the influence of a particular polymer mixture was studied, which turned out to be the best system if both a high efficiency and a low tendency to form an L(alpha) phase are needed
Description:Date Completed 17.04.2007
Date Revised 20.09.2005
published: Print
Citation Status PubMed-not-MEDLINE
ISSN:1520-5827