Adsorption of trinitrotoluene on uncoated silicon microcantilever surfaces

We measured the adsorption characteristics of trinitrotoluene (TNT) on piezoresistive silicon microcantilever surfaces under ambient air using a well-characterized TNT vapor generator. This allowed us to quantify the adsorption parameters and to estimate the sticking coefficient. The sticking coeffi...

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Bibliographische Detailangaben
Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1985. - 20(2004), 7 vom: 30. März, Seite 2690-4
1. Verfasser: Pinnaduwage, L A (VerfasserIn)
Weitere Verfasser: Yi, D, Tian, F, Thundat, T, Lareau, R T
Format: Aufsatz
Sprache:English
Veröffentlicht: 2004
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article Research Support, U.S. Gov't, Non-P.H.S. Trinitrotoluene 118-96-7 Silicon Z4152N8IUI
Beschreibung
Zusammenfassung:We measured the adsorption characteristics of trinitrotoluene (TNT) on piezoresistive silicon microcantilever surfaces under ambient air using a well-characterized TNT vapor generator. This allowed us to quantify the adsorption parameters and to estimate the sticking coefficient. The sticking coefficient initially increases with TNT exposure time and then levels off around 0.3. Atomic force microscopy images of silicon surfaces exposed to TNT revealed "island" formation of the adsorbate on the silicon surface. At low exposure times, mainly the number density of islands increased with exposure time; at longer exposure times, the size (in particular, height) of the islands grew, corresponding to the higher sticking coefficients. These observations can be qualitatively explained via the difference between TNT-surface and TNT-TNT interactions mediated by water molecules
Beschreibung:Date Completed 20.06.2005
Date Revised 26.10.2019
published: Print
Citation Status MEDLINE
ISSN:1520-5827