Deterioration Behavior of Steel Passivation Films in a Nano Perspective : Effect of Shear Stress

Corrosion of reinforcement is one of the key problems affecting the durability of concrete structures. This phenomenon begins with the deterioration of the passivation film. Regrettably, the underlying microscopic mechanisms governing the deterioration process of passivation films under stress remai...

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Publié dans:Langmuir : the ACS journal of surfaces and colloids. - 1985. - 41(2025), 39 vom: 07. Okt., Seite 26738-26750
Auteur principal: Wu, Shenrong (Auteur)
Autres auteurs: Wang, Yihan, Liu, Chengbo, Hou, Dongshuai, Zhou, Xiangming, Wang, Muhan
Format: Article en ligne
Langue:English
Publié: 2025
Accès à la collection:Langmuir : the ACS journal of surfaces and colloids
Sujets:Journal Article
Description
Résumé:Corrosion of reinforcement is one of the key problems affecting the durability of concrete structures. This phenomenon begins with the deterioration of the passivation film. Regrettably, the underlying microscopic mechanisms governing the deterioration process of passivation films under stress remain inadequately investigated. In this study, we employ molecular dynamics (MD) simulations to model the deterioration of passivation films with different defects and subjected to varying shear stresses. Notably, the presence of defects considerably compromises the passivation film's shear stress resistance. Conversely, the ideal passivation film exhibits robustness against shear stress, manifesting deformation only under high-stress conditions. Moreover, we observe that the defective film only maintains partial stability by dislocation sliding under low stress in the actual simulation. Nevertheless, as stress levels escalate, the dislocation sliding mechanism ceases to be effective, leading to interlayer deterioration and overall deterioration of the structure
Description:Date Revised 07.10.2025
published: Print-Electronic
Citation Status PubMed-not-MEDLINE
ISSN:1520-5827
DOI:10.1021/acs.langmuir.5c03130