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250829s2025 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202502393
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|a eng
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|a Tan, Xiaoyu
|e verfasserin
|4 aut
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| 245 |
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|a Design of a Tunable, High-performance Mixed Matrix Membrane Platform for Gas Separations
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|c 2025
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 28.08.2025
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2025 Wiley‐VCH GmbH.
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|a Membrane technology offers substantial economic and environmental benefits for energy-intensive chemical separations. Chabazite-type zeolite, possessing a 3-D channel system with molecular-sieving windows, can be an ideal membrane material, but conditions to synthesize zeolite-only membranes limit optimization strategies. Guided by advanced quantum chemistry calculations on inner-pore molecular interactions, zeolite properties are tailored for different separations and optimized particles incorporated in polyimide at very high loadings. A membrane platform is thus created that largely outperforms state-of-the-art membranes for a broad variety of industry-relevant applications, that is, carbon capture, natural gas/biogas purification, hydrocarbon, helium and hydrogen recovery. Accurate size-sieving of gas molecules is realized together with rational determination of optimal gas-zeolite interactions. Crucial for industrial applications, these well-tuned membranes displayed excellent non-aging properties, high flexibility and higher mixed-gas selectivities than ideal-gas selectivities. Moreover, they performed even better at low CO2-partial pressure in CO2-removal and can be made humidity-insensitive
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|a Journal Article
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|a gas separations
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|a high‐resolution molecular sieving
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|a mixed matrix membrane
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|a non‐aging
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|a tunable chemical interactions
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|a Robijns, Sven
|e verfasserin
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|a Lamaire, Aran
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|a Goeminne, Ruben
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|a De Witte, Niels
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|a Dickmann, Marcel
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|a Verbeke, Rhea
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|a Van der Donck, Tom
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|a de Oliveira Silva, Rodrigo
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|a Ke, Quanli
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|a Li, Yun
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|a Aslam, Imran
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|a Van Goethem, Cédric
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|a Donckels, Thibaut
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|a Helm, Ricardo
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|a Sakellariou, Dimitrios
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|a Van Assche, Tom
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|a Van Speybroeck, Veronique
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|a Dusselier, Michiel
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|a Vankelecom, Ivo F J
|e verfasserin
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 37(2025), 34 vom: 15. Aug., Seite e2502393
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnas
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|g volume:37
|g year:2025
|g number:34
|g day:15
|g month:08
|g pages:e2502393
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