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241223s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202417691
|2 doi
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|a pubmed25n1272.xml
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|a (DE-627)NLM381999262
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|a (NLM)39713921
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Kuang, Yazhuo
|e verfasserin
|4 aut
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| 245 |
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|a Matching P- and N-type Organic Electrochemical Transistor Performance Enables a Record High-gain Complementary Inverter
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|c 2024
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Revised 23.12.2024
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|a published: Print-Electronic
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|a Citation Status Publisher
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|a © 2024 Wiley‐VCH GmbH.
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|a The charge transport of channel materials in n-type organic electrochemical transistors (OECTs) is greatly limited by the adverse effects of electrochemical doping, posing a long-standing puzzle for the community. Herein, an n-type conjugated polymer with glycolated side chains (n-PT3) is introduced. This polymer can adapt to electrochemical doping and create more organized nanostructures, mitigating the adverse effects of electrochemical doping. This unique characteristic gives n-PT3 excellent charge transport in the doped state and reversible ion storage, making it highly suitable as an n-type organic mixed ionic-electronic conducting (OMIEC) material. n-PT3 exhibits a high electron mobility of µ ≈ 1.0 cm2 V-1 s-1 and a figure of merit value of µC* ≈ 100 F cm-1 V-1 s-1, representing one of the best results for n-type OMIEC materials. A new p-type OMIEC polymer has been synthesized as the channel material for constructing a complementary inverter to match the n-type OECT channel layer based on n-PT3. As a result, a voltage gain value of up to 307 VV-1 has been achieved, which is a record value for sub-1 V complementary inverters based on OECTs. This work offers valuable insights into designing electrochemical doping adaptive n-type OMIEC materials and fabricating high-gain organic complementary inverters
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|a Journal Article
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|a Inverter
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|a N‐type conjugated polymers
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|a electrochemical Doping
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|a mixed Ionic‐electronic Conductor
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|a organic electrochemical transistors
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|a Yao, Tangqing
|e verfasserin
|4 aut
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| 700 |
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|a Deng, Sihui
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Dong, Jingjin
|e verfasserin
|4 aut
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| 700 |
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|a Ye, Gang
|e verfasserin
|4 aut
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| 700 |
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|a Zhang, Linlong
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Shao, Shuyan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhu, Zhongjie
|e verfasserin
|4 aut
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| 700 |
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|a Liu, Jun
|e verfasserin
|4 aut
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| 700 |
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|a Liu, Jian
|e verfasserin
|4 aut
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| 773 |
0 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g (2024) vom: 23. Dez., Seite e2417691
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnas
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| 773 |
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|g year:2024
|g day:23
|g month:12
|g pages:e2417691
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|u http://dx.doi.org/10.1002/adma.202417691
|3 Volltext
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