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241015s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202411291
|2 doi
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|a pubmed25n1262.xml
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|a eng
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|a Wei, Jia-Hao
|e verfasserin
|4 aut
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|a Light-Operated Diverse Logic Gates Enabled by Modulating Time-Dependent Fluorescence of Dissipative Self-Assemblies
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|c 2024
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|a Text
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 05.12.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2024 Wiley‐VCH GmbH.
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|a Light-fueled dissipative self-assembly possesses enormous potential in the field of optical information due to controllable time-dependent optical signals, but remains a great challenge for constructing intelligent light-operated logic circuits due to the limited availability of optical signal inputs and outputs. Herein, a series of light-fueled dissipative self-assembly systems with variable optical signals are reported to realize diverse logic gates by modulating time-dependent fluorescence variations of the loaded fluorophores. Three kinds of alkyl trimethylammonium homologs are employed to co-assemble with a merocyanine-based photoinduced amphiphile separately to construct a series of dissipative self-assemblies, showing unexpectedly different fluorescence control behaviors of loaded fluorophores during light irradiation and thermal relaxation processes. The opposite monotonicity of time-dependent emission intensity is achieved just by changing the excitation wavelength. Furthermore, by varying the types of trimethylammoniums and excitation wavelengths, a robust logic system is accomplished, integrating AND, XNOR, and XOR functions, which provides an effective pathway for advancing information transmission applications
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|a Journal Article
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|a dissipative self‐assembly
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|a fluorescence control
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|a logic gate
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|a supramolecular nanoparticle
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| 700 |
1 |
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|a Xing, Junfei
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Hou, Xiao-Fang
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Chen, Xu-Man
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Li, Quan
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 49 vom: 14. Dez., Seite e2411291
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnas
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| 773 |
1 |
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|g volume:36
|g year:2024
|g number:49
|g day:14
|g month:12
|g pages:e2411291
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| 856 |
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|u http://dx.doi.org/10.1002/adma.202411291
|3 Volltext
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