Treatment of tetracycline in an aqueous solution with an iron-biochar/periodate system : Influencing factors and mechanisms

© 2024 The Authors This is an Open Access article distributed under the terms of the Creative Commons Attribution Licence (CC BY-NC-ND 4.0), which permits copying and redistribution for non-commercial purposes with no derivatives, provided the original work is properly cited (http://creativecommons....

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Veröffentlicht in:Water science and technology : a journal of the International Association on Water Pollution Research. - 1986. - 89(2024), 12 vom: 16. Juni, Seite 3344-3356
1. Verfasser: Xu, Shuo (VerfasserIn)
Weitere Verfasser: Wei, Hongyan, Li, Xuejiao, Chen, Lizhu, Song, Tiehong
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Water science and technology : a journal of the International Association on Water Pollution Research
Schlagworte:Journal Article advanced oxidation process modified biochar periodate potassium pertechnetate tetracycline Tetracycline F8VB5M810T Iron E1UOL152H7 mehr... Charcoal 16291-96-6 biochar Water Pollutants, Chemical Reactive Oxygen Species Anti-Bacterial Agents potassium ferrate 39469-86-8 Potassium Compounds Iron Compounds
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245 1 0 |a Treatment of tetracycline in an aqueous solution with an iron-biochar/periodate system  |b Influencing factors and mechanisms 
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520 |a © 2024 The Authors This is an Open Access article distributed under the terms of the Creative Commons Attribution Licence (CC BY-NC-ND 4.0), which permits copying and redistribution for non-commercial purposes with no derivatives, provided the original work is properly cited (http://creativecommons.org/licenses/by-nc-nd/4.0/). 
520 |a In this study, a potassium ferrate (K2FeO4)-modified biochar (Fe-BC) was prepared and characterized. Afterwards, Fe-BC was applied to activated periodate (PI) to degrade tetracycline (TC), an antibiotic widely used in animal farming. The degradation effects of different systems on TC were compared and the influencing factors were investigated. In addition, several reactive oxygen species (ROS) generated by the Fe-BC/PI system were identified, and TC degradation pathways were analyzed. Moreover, the reuse performance of Fe-BC was evaluated. The results exhibited that the Fe-BC/PI system could remove almost 100% of TC under optimal conditions of [BC] = 1.09 g/L, initial [PI] = 3.29 g/L, and initial [TC] = 20.3 mg/L. Cl-, HCO3-, NO3-, and humic acid inhibited TC degradation to varying degrees in the Fe-BC/PI system due to their quenching effects on ROS. TC was degraded into intermediates and even water and carbon dioxide by the synergistic effect of ROS generated and Fe on the BC surface. Fe-BC was reused four times, and the removal rate of TC was still maintained above 80%, indicating the stable nature of Fe-BC 
650 4 |a Journal Article 
650 4 |a advanced oxidation process 
650 4 |a modified biochar 
650 4 |a periodate 
650 4 |a potassium pertechnetate 
650 4 |a tetracycline 
650 7 |a Tetracycline  |2 NLM 
650 7 |a F8VB5M810T  |2 NLM 
650 7 |a Iron  |2 NLM 
650 7 |a E1UOL152H7  |2 NLM 
650 7 |a Charcoal  |2 NLM 
650 7 |a 16291-96-6  |2 NLM 
650 7 |a biochar  |2 NLM 
650 7 |a Water Pollutants, Chemical  |2 NLM 
650 7 |a Reactive Oxygen Species  |2 NLM 
650 7 |a Anti-Bacterial Agents  |2 NLM 
650 7 |a potassium ferrate  |2 NLM 
650 7 |a 39469-86-8  |2 NLM 
650 7 |a Potassium Compounds  |2 NLM 
650 7 |a Iron Compounds  |2 NLM 
700 1 |a Wei, Hongyan  |e verfasserin  |4 aut 
700 1 |a Li, Xuejiao  |e verfasserin  |4 aut 
700 1 |a Chen, Lizhu  |e verfasserin  |4 aut 
700 1 |a Song, Tiehong  |e verfasserin  |4 aut 
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773 1 8 |g volume:89  |g year:2024  |g number:12  |g day:16  |g month:06  |g pages:3344-3356 
856 4 0 |u http://dx.doi.org/10.2166/wst.2024.196  |3 Volltext 
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