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231227s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202307265
|2 doi
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|a pubmed24n1366.xml
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|a (DE-627)NLM366175815
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|a (NLM)38126918
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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| 100 |
1 |
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|a Park, Keonwoo
|e verfasserin
|4 aut
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| 245 |
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|a Atmospheric Humidity Underlies Irreproducibility of Formamidinium Lead Iodide Perovskites
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|c 2024
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Revised 04.04.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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| 520 |
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|a © 2023 Wiley‐VCH GmbH.
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|a Metal halide perovskite solar cells (PSCs) are infamous for their batch-to-batch and lab-to-lab irreproducibility in terms of stability and performance. Reproducible fabrication of PSCs is a critical requirement for market viability and practical commercialization. PSC irreproducibility plagues all levels of the community; from institutional research laboratories, start-up companies, to large established corporations. In this work, the critical function of atmospheric humidity to regulate the crystallization and stabilization of formamidinium lead triiodide (FAPbI3) perovskites is unraveled. It is demonstrated that the humidity content during processing induces profound variations in perovskite stoichiometry, thermodynamic stability, and optoelectronic quality. Almost counterintuitively, it is shown that the presence of humidity is perhaps indispensable to reproduce phase-stable and efficient FAPbI3-based PSCs
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|a Journal Article
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4 |
|a crystallizations
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4 |
|a halide perovskites
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| 650 |
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4 |
|a humidity
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| 650 |
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4 |
|a in situ studies
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| 650 |
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4 |
|a reproducibility
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| 650 |
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|a scalability
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4 |
|a solar cells
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| 650 |
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4 |
|a stability
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|a Tan, Shaun
|e verfasserin
|4 aut
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|a Kodalle, Tim
|e verfasserin
|4 aut
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| 700 |
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|a Lee, Do-Kyoung
|e verfasserin
|4 aut
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1 |
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|a Abdelsamie, Maged
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Park, Ji-Sang
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Lee, Joo-Hong
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Jung, Sung-Kwang
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Ko, Jeong Hoon
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Park, Nam-Gyu
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Sutter-Fella, Carolin M
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Yang, Yang
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Lee, Jin-Wook
|e verfasserin
|4 aut
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| 773 |
0 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 14 vom: 01. Apr., Seite e2307265
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
1 |
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|g volume:36
|g year:2024
|g number:14
|g day:01
|g month:04
|g pages:e2307265
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|u http://dx.doi.org/10.1002/adma.202307265
|3 Volltext
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