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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202209628
|2 doi
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|a pubmed24n1166.xml
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|a (DE-627)NLM349923728
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|a (NLM)36480021
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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| 100 |
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|a Li, Linlin
|e verfasserin
|4 aut
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|a Novel Insight into Rechargeable Aluminum Batteries with Promising Selenium SulfideCarbon Nanofibers Cathode
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|c 2023
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Completed 24.02.2023
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|a Date Revised 24.02.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2022 Wiley-VCH GmbH.
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|a Due to the unique electronic structure of aluminum ions (Al3+ ) with strong Coulombic interaction and complex bonding situation (simultaneously covalent/ionic bonds), traditional electrodes, mismatching with the bonding orbital of Al3+ , usually exhibit slow kinetic process with inferior rechargeable aluminum batteries (RABs) performance. Herein, to break the confinement of the interaction mismatch between Al3+ and the electrode, a previously unexplored Se2.9 S5.1 -based cathode with sufficient valence electronic energy overlap with Al3+ and easily accessible structure is potentially developed. Through this new strategy, Se2.9 S5.1 encapsulated in multichannel carbon nanofibers with free-standing structure exhibits a high capacity of 606 mAh g-1 at 50 mA g-1 , high rate-capacity (211 mAh g-1 at 2.0 A g-1 ), robust stability (187 mAh g-1 at 0.5 A g-1 after 3,000 cycles), and enhanced flexibility. Simultaneously, in/ex-situ characterizations also reveal the unexplored mechanism of Sex Sy in RABs
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|a Journal Article
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|a free-standing structures
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|a interaction bonds
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|a nanofibers
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|a rechargeable aluminum batteries
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|a selenium sulfide
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|a Ma, Yanchen
|e verfasserin
|4 aut
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|a Cui, Fangyan
|e verfasserin
|4 aut
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|a Li, Yan
|e verfasserin
|4 aut
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|a Yu, Deshuang
|e verfasserin
|4 aut
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|a Lian, Xintong
|e verfasserin
|4 aut
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|a Hu, Yuxiang
|e verfasserin
|4 aut
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|a Li, Hongyi
|e verfasserin
|4 aut
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|a Peng, Shengjie
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 8 vom: 08. Feb., Seite e2209628
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:35
|g year:2023
|g number:8
|g day:08
|g month:02
|g pages:e2209628
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|u http://dx.doi.org/10.1002/adma.202209628
|3 Volltext
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