MnO2 Synergized with N/S Codoped Graphene as a Flexible Cathode Efficient Electrocatalyst for Advanced Honeycomb-Shaped Stretchable Aluminum-Air Batteries

Aluminum-air batteries possess high theoretical specific capacities and energy densities. However, the desired application performance in the field of flexible electronics is limited by the rigid battery structure and slow kinetics of the oxygen reduction reaction (ORR). To address these issues, fle...

Ausführliche Beschreibung

Bibliographische Detailangaben
Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1992. - 36(2020), 43 vom: 03. Nov., Seite 12954-12962
1. Verfasser: Shui, Ziyi (VerfasserIn)
Weitere Verfasser: Liao, Xiangbiao, Lei, Yuan, Ni, Jia, Liu, Yilun, Dan, Yong, Zhao, Wei, Chen, Xi
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article
LEADER 01000naa a22002652 4500
001 NLM316688347
003 DE-627
005 20231225161629.0
007 cr uuu---uuuuu
008 231225s2020 xx |||||o 00| ||eng c
024 7 |a 10.1021/acs.langmuir.0c02246  |2 doi 
028 5 2 |a pubmed24n1055.xml 
035 |a (DE-627)NLM316688347 
035 |a (NLM)33100011 
040 |a DE-627  |b ger  |c DE-627  |e rakwb 
041 |a eng 
100 1 |a Shui, Ziyi  |e verfasserin  |4 aut 
245 1 0 |a MnO2 Synergized with N/S Codoped Graphene as a Flexible Cathode Efficient Electrocatalyst for Advanced Honeycomb-Shaped Stretchable Aluminum-Air Batteries 
264 1 |c 2020 
336 |a Text  |b txt  |2 rdacontent 
337 |a ƒaComputermedien  |b c  |2 rdamedia 
338 |a ƒa Online-Ressource  |b cr  |2 rdacarrier 
500 |a Date Revised 03.11.2020 
500 |a published: Print-Electronic 
500 |a Citation Status PubMed-not-MEDLINE 
520 |a Aluminum-air batteries possess high theoretical specific capacities and energy densities. However, the desired application performance in the field of flexible electronics is limited by the rigid battery structure and slow kinetics of the oxygen reduction reaction (ORR). To address these issues, flexible, stretchable, and customizable aluminum-air batteries with a reference to honeycomb shape are composed of multilayer single battery units to achieve large scalability and start-stop control. The single aluminum-air battery combines MnO2 with N/S codoped graphene to improve the electrocatalytic activity. Benefiting from an efficient electrocatalyst and reasonable structural design, the single aluminum-air battery exhibits excellent electrochemical characteristics under deformation conditions with a high specific capacity and energy density (1203.2 mAh g-1 Al and 1630.1 mWh g-1 Al). Furthermore, the obtained honeycomb-shaped stretchable aluminum-air batteries maintain a stable output voltage over the 2500% stretching. More interestingly, the stretchable honeycomb structure not only can solve the start-stop control problem but also has the potential to reduce the self-corrosion in disposable metal-air batteries. In addition, owing to the customizable shapes and sizes, the honeycomb-shaped stretchable aluminum-air batteries facilitate the integrated application of flexible batteries in wearables 
650 4 |a Journal Article 
700 1 |a Liao, Xiangbiao  |e verfasserin  |4 aut 
700 1 |a Lei, Yuan  |e verfasserin  |4 aut 
700 1 |a Ni, Jia  |e verfasserin  |4 aut 
700 1 |a Liu, Yilun  |e verfasserin  |4 aut 
700 1 |a Dan, Yong  |e verfasserin  |4 aut 
700 1 |a Zhao, Wei  |e verfasserin  |4 aut 
700 1 |a Chen, Xi  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Langmuir : the ACS journal of surfaces and colloids  |d 1992  |g 36(2020), 43 vom: 03. Nov., Seite 12954-12962  |w (DE-627)NLM098181009  |x 1520-5827  |7 nnns 
773 1 8 |g volume:36  |g year:2020  |g number:43  |g day:03  |g month:11  |g pages:12954-12962 
856 4 0 |u http://dx.doi.org/10.1021/acs.langmuir.0c02246  |3 Volltext 
912 |a GBV_USEFLAG_A 
912 |a SYSFLAG_A 
912 |a GBV_NLM 
912 |a GBV_ILN_22 
912 |a GBV_ILN_350 
912 |a GBV_ILN_721 
951 |a AR 
952 |d 36  |j 2020  |e 43  |b 03  |c 11  |h 12954-12962