Well-Designed Porous Graphene Flakes for Lithium-Ion Batteries with Outstanding Rate Performance

Porous graphene flakes (PGFs) with controllable pore sizes are selectively prepared through self-assembly of Fe3O4 nanoparticles on organic modified montmorillonite combined with carbonization and subsequent annealing treatment. The resulting PGFs with a thickness of 5 nm have a specific surface are...

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Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1985. - 35(2019), 39 vom: 01. Okt., Seite 12613-12619
1. Verfasser: Kukułka, Wojciech (VerfasserIn)
Weitere Verfasser: Kierzek, Krzysztof, Stankiewicz, Natalia, Chen, Xuecheng, Tang, Tao, Mijowska, Ewa
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2019
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article
Beschreibung
Zusammenfassung:Porous graphene flakes (PGFs) with controllable pore sizes are selectively prepared through self-assembly of Fe3O4 nanoparticles on organic modified montmorillonite combined with carbonization and subsequent annealing treatment. The resulting PGFs with a thickness of 5 nm have a specific surface area of 337 m2/g, pore volume of 0.66 cm3/g, and mean pore diameter of 15 nm. Due to their unique porous flake structures, PGFs show an impressive rate performance in lithium-ion batteries, especially at high current densities (238 mA h/g at 10 C) as well as long-term stability in comparison to the commercial graphite (55 mA h/g at 10 C). Therefore, PGFs with their key structural properties serve as ideal candidates as electrode components in lithium-ion batteries and show great potential application in other energy storage fields
Beschreibung:Date Revised 04.03.2020
published: Print-Electronic
Citation Status PubMed-not-MEDLINE
ISSN:1520-5827
DOI:10.1021/acs.langmuir.8b03477