Gaseous adsorption in melanins : hydrophilic biomacromolecules with high electrical conductivities

The melanins are an important class of multifunctional biomacromolecules that possess a number of intriguing physical and chemical properties including electrical and photoconductivity. Unusually for a conducting organic material, eumelanin is hydrophilic and its electrical properties are strongly d...

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Détails bibliographiques
Publié dans:Langmuir : the ACS journal of surfaces and colloids. - 1985. - 26(2010), 1 vom: 05. Jan., Seite 412-6
Auteur principal: Mostert, A Bernardus (Auteur)
Autres auteurs: Davy, Karl J P, Ruggles, Jeremy L, Powell, Ben J, Gentle, Ian R, Meredith, Paul
Format: Article en ligne
Langue:English
Publié: 2010
Accès à la collection:Langmuir : the ACS journal of surfaces and colloids
Sujets:Journal Article Research Support, Non-U.S. Gov't Gases Melanins Water 059QF0KO0R eumelanin 12627-86-0 Ethanol 3K9958V90M
Description
Résumé:The melanins are an important class of multifunctional biomacromolecules that possess a number of intriguing physical and chemical properties including electrical and photoconductivity. Unusually for a conducting organic material, eumelanin is hydrophilic and its electrical properties are strongly dependent on its hydration state. We have therefore measured adsorption isotherms for two polar adsorbates, water and ethanol, in the pressed powder pellets of synthetic eumelanin typically used in electrical studies. We show that a simple kinetic monolayer Langmuir model describes the adsorption and find that there are strong adsorbate-eumelanin interactions in both cases. These isotherms allow the proper scaling of electrical conductivity data and in doing so make progress toward a better understanding of eumelanin electrical properties, which is a critical prerequisite to the design of new eumelanin-like bioelectronic materials
Description:Date Completed 02.03.2010
Date Revised 21.11.2013
published: Print
Citation Status MEDLINE
ISSN:1520-5827
DOI:10.1021/la901290f